Summary of Research Project Results Under the JSPS FY2000
"Research for the future Program"



1.Research Institution@Tokyo Institute of Technology
@
2.University-Industry Cooperative Research Committee@69th Committee on Materials Processing and Applications
@
3.Term of Project@FY1996`FY2000
@
4.Project Number@96R06901
@
5.Title of Project@Preparation of Advanced Inorganic Materials by Soft Solution Processing

6.Projetct Leader
Name Institution,Department Title of Position
Masahiro Yoshimura Tokyo Institute of Technology, Materials and Structure Laboratory Professor

7.Core Members

Names Institution,Department Title of Position
Yusuke Moriyoshi Hosei University, Faculty of Engineering Professor
Yasumichi Matsumoto Kumamoto University, Faculty of Engineering Professor
masanori Abe Tokyo Institute of Technology, Graduate School of Science and Engineering Professor

8.Cooperating Researchers

Names Institution,Department Title of Position
Kazunari Domen Tokyo Institute of Technology, Chemical Resources Laboratory Professor
Masato Kakihana Tokyo Institute of Technology, Materials and Structure Laboratory Associate Professor
Kiyoshi Okada Tokyo Institute of Technology, Graduate School of Science and Engineering Professor

9.Summary of Research Results

We have succeeded in the following results:
1. Direct fabrication of Li-double oxide films by electrochemical methods.
2. Direct fabrication of Li-double oxide films by hydrothermal methods.
3. BaTiO3/SrTiO3 films by electrochemical/hydrothermal ethods.
4. Layered BaTiO3/SrTiO3 films in flow-type hydrothermal/electrochemical cell.
5. Direct laser patterning of BaTiO3, SrTiO3 films in solutions.
6. Direct patterning of LiCoO2 by electrochemical method.
7. Direct patterning of Cds, PbS film by ink jet.
8. Hydrothermal synthesis of carbon nanotubes nanocells.
9. High purity synthesis of LiMnO3, BaTiO3, LiTaO3, etc., by polymerized complex methods.
10. Fabrication of new photo catalysis by polymerized complex method.
11. Preparation and characterization of various ferrite films by ferrite plating.
12. Ultrasonically assisted ferrite plating of ferrite on polymer globules.
13. Direct fabrication of porous apatite.
14. Layered PbO2/TiO2 film by electrochemical deposition.
15. Fixiation of CO2 by CaSiO3 with SiO2 production.
These results have been published in >300 papers and 12 patents, and several international symposia. Our project can be concluded to be quite successful.

10.Key Words

(1)Soft ProcessA(2)Solution ProcessA(3)Films
(4)CeramicsA(5)PatterningA(6)Porous Materials
(7)BaTiO3A(8)LiCoO2A(9)Carbon

11.References

[Reference Articles]
Author Title of Article
Masato Kakihana Polymerized Complex Route to the Synthesis of Pure YsTi2O7 at 750 Ž Using Y:Ti Mixed-Metal Citric Acid Complex
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 79[6] 1996 1673-1676

Author Title of Article
Woo-Seok Cho and Masahiro Yoshimura Preparation of highly crystallized BaMoO4 film using a solution reaction assisted by electrochemical dissolution of molybdenum
Journal Volume Year Pages Concerned
Solid State Ionics 100 1997 143-147

Author Title of Article
Woo-Seok Cho and Masahiro Yoshimura Structure evolution of highly crystallized BaWO4 film prepared by an electrochemical method at room temperature
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 80[9] 1997 2199-2204

Author Title of Article
Masahiro Yoshimura, Masato Kakihana, et al Preparation and luminescence of crystallized Ba1-xSrxMoO4 solid-solution films by an electrochemical method at room temperature
Journal Volume Year Pages Concerned
Jpn. J. Appl. Phys. 36 1997 L1229-1231

Author Title of Article
Woo-Seok Cho and Masahiro Yoshimura Characterization of Ba1-xSrxWO4 solid-solution films prepared by an electrochemical method at room temperature
Journal Volume Year Pages Concerned
Jpn. J. Appl. Phys. 36 1997 5658-5662

Author Title of Article
Masahiro Yoshimura, Masato Kakihana, et al Preparation of crystallized Sr1-xCaxMoO4 solid-solution films by an electrochemical method at room temperature and their luminescence
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 80[9] 1997 2464-2466

Author Title of Article
Woo-Seok Cho and Masahiro Yoshimura Structural evolution of crystallized SrWO4 film synthesized by a solution reaction assisted by electrochemical dissolution of tungsten at room temperature
Journal Volume Year Pages Concerned
Eur. J. Solid State Inorg. Chem. t.34 1997 895-904

Author Title of Article
Woo-Seok Cho, Masahiro Yoshimura, et al Active electrochemical dissolution of molybdenum and application for room-temperature synthesis of crystallized luminescent calcium molybdate film
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 80[3] 1997 765-769

Author Title of Article
Masahiro Yoshimura and Wojciech Suchanek In situ fabrication of morphology-controlled advanced ceramic materials by Soft Solution Processing
Journal Volume Year Pages Concerned
Solid State Ionics 98 1997 197-208

Author Title of Article
Wojciech Suchanek, Masahiro Yoshimura, et al Hydroxyapatite ceramics with selected sintering additives
Journal Volume Year Pages Concerned
Biomaterials 18[13] 1997 923-933

Author Title of Article
Masato kakihana, Masahiro Yoshimura, et al Polymerized Complex Synthesis of perovskite lead titanate at reduced temperatures: possible formation of heterometallic (Pb, Ti) -Citric Aced Complex
Journal Volume Year Pages Concerned
Chem. Mater. 9 1997 451-456

Author Title of Article
Masatomo Yashima, Masahiro Yoshimura, et al Crystallization of hafnia and zirconia during the pyrolysis of acetate gels
Journal Volume Year Pages Concerned
J. Mater. Res. 12[10] 1997 2575-2583

Author Title of Article
Masatomo Yashima, Masahiro Yoshimura, et al Raman spectral characterization of existing phases in the Y2O3-Nb2O5 system
Journal Volume Year Pages Concerned
J. Phys. Chem. Solids 58[10] 1997 1593-1597

Author Title of Article
Wojciech Suchabnek, Masahiro Yoshimura, et al Hydroxyapatite/hydroxyapatite-whisker composites without sintering additives: mechanical properties and microstructural evolution
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 80[11] 1997 2805-2813

Author Title of Article
Masato Kakihana, Masahiro Yoshimura, et al Polymerized Complex Synthesis of pure perovskite PbTiO3 powders at 400-600 Ž using Pb: Ti mixed-metal citric aced complex
Journal Volume Year Pages Concerned
Chem. Mater. 9 1997 451-456

Author Title of Article
Masato Kakihana Polymerized Complex Synthesis of nanocomposite BaTi4O9/RuO2 photo-catalytic materials
Journal Volume Year Pages Concerned
Mater. Res. Soc. Symposium Proceedings 457 1997 323-334

Author Title of Article
Y. Kitamoto, M. Naoe, et al Sputter-deposition of Co-Cr-Ta Alloy Layers on Ni-Zn Ferrite Plated Underlayers
Journal Volume Year Pages Concerned
IEEE Trans. Mgn. 33[5] 1997 3085-3087

Author Title of Article
Yoshitaka Kitamoto, Masanori Abe, et al Ferrite-plated thin filmf sor perpendicular recording media
Journal Volume Year Pages Concerned
J. Mag. Soc. Jpn. 21[S2] 1997 81-84

Author Title of Article
Minjuan Zhang, Masanori Abe, et al Ultrasonic visualization of still and flowing waters using contrast agents of magnetite-encapsulates porous silica microspheres
Journal Volume Year Pages Concerned
Jpn. J. Appl. Phys. 36[1A] 1997 243-246

Author Title of Article
Y. Matsumoto, et al electrochemical behavior of Ln-Ni-oxide/Pt electrode in alkaline solution
Journal Volume Year Pages Concerned
J. Electroanal. Chem. 434 1997 235-237

Author Title of Article
Michio Koinuma, Y. Matsumoto, et al Electrochemical preparation of cobalt oxide using an autoclave electrolytic cell
Journal Volume Year Pages Concerned
J. Mater. Res. 13[4] 1998 837-839

Author Title of Article
Wojciech Suchanek and Masahiro Yoshimura Preparation of fibrous porous hydroxyapatite ceramics from hydroxyapatite whiskters
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 81[3] 1998 765-767

Author Title of Article
Wojciech Suchanek and Masahiro Yoshimura Processing and properties of hydroxyapatite-based biomaterials for use as hard tissue replacement implants
Journal Volume Year Pages Concerned
J. Mater. Res. 13[1] 1998 94-117

Author Title of Article
Masahiro Yoshimura, Masato Kakihan, et al Low-temperature synthesis of crystallized Ca1-xSrxTiO3 solid-solution films on titanium substrates by a modified hydrothermal-electrochemicdal technique
Journal Volume Year Pages Concerned
J. Alloys and Compounds 265 1998 132-136

Author Title of Article
Masahiro Yoshimura Important of Soft Solution Processing for Advanced Inorganic Materials
Journal Volume Year Pages Concerned
Journal of Materials Research 13[4] 1998 796-802

Author Title of Article
M. Yoshimura Functionally Graded SrTiO3-BaTiO3 Thin Films Prepared by The Hydrothermal-Electrochemical Method under Flowing Solution
Journal Volume Year Pages Concerned
Journal of Materials Research 13[4] 1998 875-879

Author Title of Article
Junfeng Ma Synthesis of ZrO2-Y6WO12 Solid Solution Powders by a Polymerized Complex Method
Journal Volume Year Pages Concerned
Journal of Materials Research 13[4] 1998 939-943

Author Title of Article
Masahiro Yoshimura Low-Temperature Synthesis of Crystallized Ca1-xSrxTiO3 Solid-Solution Films on Titanium Substrates by a Modified Hydrothermal-Electrochemical Technique
Journal Volume Year Pages Concerned
Journal of Alloys and Compounds 265 1998 132-136

Author Title of Article
Kyoo-Sseung Han Fabrication in a Simple Synthetic Step of Electrochemically Active LiMO2 (M=Ni and Co) Thin-Film Electrodes Using Soft Solution Processing at 20 - 200 Ž
Journal Volume Year Pages Concerned
Chemistry of Materials 10[8] 1998 2183-2188

Author Title of Article
Kyoo-Seung Han Soft Solution Processing for Fabrication of L+ithiated Thin-Film Electrodes in a Single Synthetic Step
Journal Volume Year Pages Concerned
Journa of Materials Chemistry 8[9] 1998 2403-2048

Author Title of Article
Ryu Abe, Kazunari Domen, et al Preparation of thin films of a layered titanate by the exfoliation of CsxTi(2-x/4) X/4O4
Journal Volume Year Pages Concerned
Chem. Mater. 10[1] 1998 329-333

Author Title of Article
M. Abe, H. Unuma, et al Ferric hydroxide crystal growth on arachie aced monomolecular layer spread on aqueous FeCl2 solution
Journal Volume Year Pages Concerned
J. Mag. Soc. Jpn. 22[S1] 1998 446-448

Author Title of Article
Masahiro Abe, Yoshitaka Kitamoto, et al Sonochemical surface modification of expanded polyetrafluoroethy and ferrite plating
Journal Volume Year Pages Concerned
J. Mag. Soc. Jpn. 22[S1] 1998 443-445

Author Title of Article
Yoshitaka Kitamoto, Masanori Abe, et al Fine grained Ni-Zn ferrite-plated backlayers for Co-Cr-Ta perpendicular magnetic recording media
Journal Volume Year Pages Concerned
J. Mag. Soc. Jpn. 11[S1] 1998 167-169

Author Title of Article
Michio Koinuma, Y. Matsumoto, et al Electrochemical preparation of cobalt oxide using an autoclave electrolytic cell
Journal Volume Year Pages Concerned
J. Mater. Res. 13[4] 1998 837-839

Author Title of Article
Wojciech Suchanek Processing and Properties of Hydroxyapatite-based Biomaterials for Use as Hard Tissue Replacement Implants
Journal Volume Year Pages Concerned
Journal of Materials Research 13[1] 1998 94-117

Author Title of Article
Shigeru Ikeda Preparation of K2La2Ti3O10 by Polymerized Complex Method and Photocatalytic Decomposition of Water
Journal Volume Year Pages Concerned
Chemistry of Materials 10[1] 1998 72-77

Author Title of Article
Ryu Abe A Microporous Structure of a Thin Film Made of an Ion-Exchangeable Layered Compound
Journal Volume Year Pages Concerned
Supramolecular Science 5 1998 229-233

Author Title of Article
Masanori Abe Ferric Hydroxide Crystal Growth on Arachic Acid Monomolecular Layer Spread on Aqueous FeCl2 Solution
Journal Volume Year Pages Concerned
Journal of The Magnetic Society of Japan 22[S1] 1998 446-448

Author Title of Article
Masanori Abe Sonochemical Surface Modification of Expanded Polytetra fluoroethylene and Ferrite Plating
Journal Volume Year Pages Concerned
Journal of The Magnetics Society of Japan 22[S1] 1998 443-445

Author Title of Article
Yoshitaka Kitamoto, Fine Grained Ni-Zn Ferrite-Plated Backlayers for Co-Cr-Ta Perpendicular Magnetic Recording Media
Journal Volume Year Pages Concerned
Journal of The Magnetic Society of Japan 22[S1] 1998 167-169

Author Title of Article
Judit Szanics, Preparation of LiTaO3 Powders at Reduced Temperatures by a Polymerized Complex Method
Journal Volume Year Pages Concerned
Journal of Alloys and Compounds 281 1998 206-210

Author Title of Article
Masahiro Yoshimura, Shunsuke Tsurimoto Direct fabrication of thin-film LiNiO2 electrodes in LiOH solution by electrochemical-hydrothermal method
Journal Volume Year Pages Concerned
Solid State Ionics 106 1998 39-44

Author Title of Article
Woo-Seok Cho, and Masahiro Yoshimura Structural evolution and characterization of crystallized luminescent Sr1-xCaxWO4 solid-solution films prepared by an electrochemical method at room temperature
Journal Volume Year Pages Concerned
J. Appl. Phys. 83[1] 1998 518-523

Author Title of Article
Masahiro Yoshimura Importance of soft, solution processing for advanced inorganic materials
Journal Volume Year Pages Concerned
J. Mater. Res. 13[4] 1998 796-802

Author Title of Article
Masahiro Yoshimura, Bungo Sakurai, eet al Functionally graded SrTiO3-BaTiO3 thin films prepared by the hydrothermal-electrochemical method solution with flowing solution
Journal Volume Year Pages Concerned
J. Mater. Res. 13[4] 1998 875-879

Author Title of Article
Junfent Ma, Masatomo Yashima, et al Synthesis of ZrO2-Y6WO12 solid solution powders by a Polymerized Complex Method
Journal Volume Year Pages Concerned
J. Mater. Res. 13[4] 1999 939-943

Author Title of Article
Shigeru Ikeda, Masato Kakihana, et al Preparation of K2La2Ti3O10 by Polymerized Complex Method and photocatalytic decomposition of water
Journal Volume Year Pages Concerned
Chem. Mater. 10[1] 1998 72-77

Author Title of Article
Wojciech Suchanek Solution Flow System for Hydrothermal-Electrochemical Synthesis: New Opportunities for Multilayered Oxide Films
Journal Volume Year Pages Concerned
Materials Research Society Symposium Proceeding 517 1998 639-649

Author Title of Article
Masato Kakihana Polymerized Complex Route to the Synthesis of Pure SrTiO3 at Reduced Temperatures: Implication for Formation fo Sr-Ti Heterometallic Citric Acid Complex
Journal Volume Year Pages Concerned
Journal of Sol-Gel Scienced and Technology 12 1998 95-109

Author Title of Article
Wojciech Suchanek ƒΐ-Rhenanite (ƒΐ-NaCaPO4) as Weak Interphase for Hydroxyapatite Ceramics
Journal Volume Year Pages Concerned
Journal of the European Ceramic Society 18 1998 1923-1929

Author Title of Article
Ryu Abe Preparation of Thin Films of a Layered Titanate by the Exfoliation of CSxTi(2-x/4) x/4O4
Journal Volume Year Pages Concerned
Chemistry of Materials 10[1] 1998 329-333

Author Title of Article
Ryu Abe Preparation of Ion-Exchangeable Thin Films of Layered Niobate K4Nb6O17
Journal Volume Year Pages Concerned
Chemistry of Materials 10[6] 1998 1647-1651

Author Title of Article
Ryu Abe Preparation of Porous Niobium Oxide by the Exfoliation of K4Nb6O17 and its Photocatalytic Activity
Journal Volume Year Pages Concerned
Journal of Materials Research 13[4] 1998 861-865

Author Title of Article
Masahiro Yoshimura, Direct Fabrication of Thin-Film LiNiO2 Electrodes in LiOH Solution by Electrochemical-Hydrothermal Method
Journal Volume Year Pages Concerned
Solid State Ionics 106 1998 39-44

Author Title of Article
Wojciech Suchanek, Preparation of BaTiO3 Thin Films by the Hydrothermal Electrochemical Method in the Flowing Solution
Journal Volume Year Pages Concerned
Solid State Ionics 109 1998 65-72

Author Title of Article
Masahiro Yoshimura Functional Graded SrTiO3-BaTiO3 Thin Films Prepared by the Hydrothermal-Electrochemical Method under Flowing Solution
Journal Volume Year Pages Concerned
Journal of Materials Research 13[4] 1998 875-879

Author Title of Article
Petr Krtil Electrochemical Preparation of Oxide Materials for Electrochemistry and Electronics
Journal Volume Year Pages Concerned
Journal of Solid State Electrochem 2 1998 321-327

Author Title of Article
Chandana P. Udawatte, Preparation of Pure Perovskite-type BaSnO3 Powders by the Polymerized Complex Method at Reduced Temperature
Journal Volume Year Pages Concerned
Solid State Ionics 108 1998 23-30

Author Title of Article
Woo-Seok Cho Structural Evolution and Characterization of Crystallized Luminescent Sr1-xCaxWO4 Solid-Solution Films Prepared by an Electrochemical Method at Room Temperature
Journal Volume Year Pages Concerned
Journal of Applied Physics 83[1] 1998 518-523

Author Title of Article
Yoichi Yamashita Polymerizable Complex Synthesis of RuO2/BaTi4O9 Photocatalysts at Reduced Temperatures: Factors Affecting the Photocatalytic Activity for Decomposition of Water
Journal Volume Year Pages Concerned
Chemistry of Materials 11[1] 1998 61-66

Author Title of Article
Masahiro YOSHIMURA Recent Developments in Soft, Solution Processing: One Step Fabrication of Functional double Oxide Films by Hydrothermal-Electrothermal Methods
Journal Volume Year Pages Concerned
Journal of Materials Chemistry 9[1] 1999 77-82

Author Title of Article
Kyoo-Seung HAN Simultaneous and Direct Fabrication of Lithium Cobalt Oxide Film and Powder Using Soft Solution Processing at 100 Ž
Journal Volume Year Pages Concerned
Electrochemical and Solid-State Letters 2[2] 1999 63-66

Author Title of Article
Masato KAKIHANA Spectroscopic Characterization of Precursors Used in the Pechini-Type Polymerizable Complex Processing of Barium Titanate
Journal Volume Year Pages Concerned
Chemistry of Materials 11 1999 438-450

Author Title of Article
Kyoo-Seung HAN Fabrication Temperature and Applied Current Density Effects on Direct Fabrication of Lithium Nickel Oxide Thin Film Electrodes in LiOH Solution by Electrochemical-Hydrothermal Method
Journal Volume Year Pages Concerned
Solid State Ionics 121 1999 229-233

Author Title of Article
Wojciech SUCHANEK Stability of Fullerenes under Hydrothermal Conditions
Journal Volume Year Pages Concerned
Journal of Materials Research 14[2] 1999 323-326

Author Title of Article
Y. KITAMOTO Low-temperature Fabrication of Co Ferrite Thin Films with High Coercivity for Perpendicular Recording Disks by Wet Process
Journal Volume Year Pages Concerned
Mournal of Magnetism and Magnetic Materials 193 1999 97-100

Author Title of Article
Masanoro ABE Ferrite Films Synthesized from Aqueous Solution and Their Applications
Journal Volume Year Pages Concerned
Nano-Crystalline and Thin Film Magnetic Oxides @ 1999 27-42

Author Title of Article
Michio KOINUMA Preparation of PZT Thin Films on Stainless Steel Using Electrochemical Reduction
Journal Volume Year Pages Concerned
Journal of Solid State Chemistry 136[2] 1998 293-297

Author Title of Article
Michio KOINUMA Eledctrochemical Preparation of Cobalt Oxide Using an Autoclave Electrolytic Cell
Journal Volume Year Pages Concerned
Journal of Materials Research 13[4] 1998 837-839

Author Title of Article
Yoichi Yamashita Polymerizable Complex Synthesis of RuO2/BaTi4O9 Photocatalysts at Reduced Temperatures: Factors Affecting the Photocatalytic Activity for Decomposition of Water
Journal Volume Year Pages Concerned
Chemistry of Materials 11[1] 1998 61-66

Author Title of Article
Y. KITAMOTO Low-temperature Fabrication of Co Ferrite Thin Films with High Coercivity for Perpendicular Recording Disks by Wet Process
Journal Volume Year Pages Concerned
Mournal of Magnetism and Magnetic Materials 193 1999 97-100

Author Title of Article
Yohichi YAMASHITA Polymerizable Complex Synthesis of RuO2/BaTi409 Photocatalysts at Reduced Temperatures: Factors Affecting the Photocatalytic Activity for Decomposition of Water
Journal Volume Year Pages Concerned
Chemistry of Materials 11[1] 1999 61-66

Author Title of Article
Kiyoshi OKADA Surface Acidity and Hydrophilicity of Coprecipitated A12O3SiO2 Xerogels Prepared from Aluminium Nitrate Nanohydrate and TEtraethylorthosilicate
Journal Volume Year Pages Concerned
Journal of Colloid and Interface Science 219 1999 195-200

Author Title of Article
Takeshi SUMIDA Characterization of Layered Titanate Thin Films
Journal Volume Year Pages Concerned
Electrochemistry 12 1999 1224-1226

Author Title of Article
Yasumichi MATSUMOTO Deposition of Metallic Oxides on TiO2 Electrode Using the Photoelectrochemical Epitaxial Growth Technique (PEEG), and Electrochemical Behavior of hte PbO2/TiO2 Electrode
Journal Volume Year Pages Concerned
The Journal of Physical Chemistry B 103[34] 1999 7190-7194

Author Title of Article
Y. KITAMOTO Co Ferrite Films with Excellent Perpendicular Magnetic Anisotropy and High Coercivity Deposited at Low Temperature
Journal Volume Year Pages Concerned
Journal of Applied Physics 85[8] 1999 4708-4710

Author Title of Article
M. ABE Magnetic Film Growth at 30 Ž on Organic Monomolecular Layer, Mimicking Bacterial Magnetosome Synthesis
Journal Volume Year Pages Concerned
Journal of Applied Physics 85[8] 1999 5705-5707

Author Title of Article
Zhibin WU Electrochemical Studies on the Mechanism of the Fabrication of Ceramic Films by Hydrothermal-Electrochemical Ttechnique
Journal Volume Year Pages Concerned
Bull. Korean Chemical Society 20[8] 1999 869-874

Author Title of Article
Masahiro YOSHIMURA Soft Solution Processing: Low-Energy Direct Fabrication of Advanced Inorganic Materials
Journal Volume Year Pages Concerned
Bull. Korean Chemical Society 20[8] 1999 875-878

Author Title of Article
Judit Szanics A Novel Tantalic Acif-Based Polymerizable Complex Route to LiTaO3 Using Neither Alkoxides not Chlorides of Tantalum
Journal Volume Year Pages Concerned
Chemistry of Materials 11[10] 1999 2760-2763

Author Title of Article
Masato KAKIHANA Chemical Design of Highly Water-Soluble Ti, Nb and Ta Precursors for Multi-Component Oxides
Journal Volume Year Pages Concerned
Bull. Korean Chemical Society 20[8] 1999 893-896

Author Title of Article
Masato KAKIHANA Synthesis and Characteristics of Complex Multicomponent Oxides Prepared by Polymer Complex Method
Journal Volume Year Pages Concerned
Bull. Chemical Society of Japan 72 1999 1427-1443

Author Title of Article
Hiroyuki TAKAHASHI Synthesis of NiO-loaded KTiNbO5 Photocatalysts by a Novel Polymerizable Complex Method
Journal Volume Year Pages Concerned
Journal of Alloys and Compounds 285 1999 77-81

Author Title of Article
Masahiro YOSHIMURA In situ Fabrication of SrTiO3-BaTiO3 Layered Thin Films by Hydrothermal-Electrochemical Technique
Journal Volume Year Pages Concerned
Journal of European Ceramic Society 19 1999 1353-1359

Author Title of Article
Masato KAKIHANA Synthesis of High Surface Area LaMnO3+d by a Polymerized Complex Method
Journal Volume Year Pages Concerned
Journal of Alloyes and Compounds 283 1999 102-105

Author Title of Article
Wojcieth L. SUCHANEK A Solution Flow System for Hydrothermal-Electrothermal Growth of Multilayered Thin Films
Journal Volume Year Pages Concerned
Rev. Science Instruments 70 1999 2432-2437

Author Title of Article
Masato KAKIHANA Synthesis and Characteristics of Complex Multicomponent Oxides by Polymerized Complex Method
Journal Volume Year Pages Concerned
Bull. Chemical Society of Japan @ 1999 1427-1443

Author Title of Article
Petr KRTIL Electrochemical Formation of Ternary Oxide Films-an EQCM Approach to Galvanostatic Deposition of Alkali Earth Metal Tungstates and Molybdates
Journal Volume Year Pages Concerned
Electrochimica Acta 44 1999 3911-3920

Author Title of Article
Zhibin WU Investigations on Procedures of the Fabrication fo Barium Titanate Ceramic Films under Hydrothermal-Electrochemical Conditions
Journal Volume Year Pages Concerned
Solid State Ionics 122 1999 161-172

Author Title of Article
Yoshitaka KITAMOTO Nanostructured Oxide Films by Ferrite Plating with Sonochemistry
Journal Volume Year Pages Concerned
Nano Structured Materials 12 1999 41-44

Author Title of Article
Y. KITAMOTO Intergranular Coupling and Activation Volume of Co-Ni Ferrite Thin Films with High Coercivity Above 3 kOe
Journal Volume Year Pages Concerned
IEEE Transactions on Magnetics 35[5] 1999 2694-2696

Author Title of Article
Fuchun ZHANG Spin-Spray Ferrite-Plated Co Ferrite Films with High Coercitity for Perpendicular Magnetic Recording Media
Journal Volume Year Pages Concerned
IEEE Transactions on Magnetics 35[5] 1999 2751-2753

Author Title of Article
Y. NAKAYAMA Preparation of Ferrite Films for Electrical Insulation by Ultrasound-Enhanced Ferrite Plating
Journal Volume Year Pages Concerned
IEEE Transactions on Magnetics 35[5] 1999 3040-3042

Author Title of Article
Kazuhiro NISHIMURA Electro-Ferrite Plating of Magnetite at 24-80 Ž
Journal Volume Year Pages Concerned
IEEE Transactions on Magnetics 35[5] 1999 3043-3045

Author Title of Article
Makoto OJIMA Ultrasound Enhanced Ferrite Plating of Polymer Microspheres for Magnetic Cellular Segregation
Journal Volume Year Pages Concerned
IEEE Transactions on Magnetics 35[5] 1999 4118-4120

Author Title of Article
Masanoro ABE Ferrite Films Synthesized from Aqueous Solution and Their Applications
Journal Volume Year Pages Concerned
Nano-Crystalline and Thin Film Magnetic Oxides @ 1999 27-42

Author Title of Article
S. W. SONG Effect of LiOH Concentration Change on Simultaneous Preparation of LiCoO2 Film and Powder by Hydrothermal Method
Journal Volume Year Pages Concerned
Proc. of SSI-12, Solid State Ionics 135-137 2000 277-282

Author Title of Article
Hirotaka FUJIMORI Phase Transition and Soft Phonon Modes in SrZrO3 around 1200 Ž by Ultraviolet Laser Raman Spectroscopy
Journal Volume Year Pages Concerned
Physical Review B 61 2000 3971-3974

Author Title of Article
Hirotaka FUJIMORI In situ Observation of Defects in Hydroxyapatite up to 1200C by Ultraviolet Raman Spectroscopy
Journal Volume Year Pages Concerned
Chem. Phy. Lett 325 2000 383-388

Author Title of Article
Jose M. CALDERON-MORENO Carbon Nanocells and Nanotubes Grown in Hydrothermal Fluids
Journal Volume Year Pages Concerned
Chem. Phys. Lett 329 2000 317-322

Author Title of Article
Masahiro YOSHIMURA Soft Solution-processing-A Strategy for One-Step Processing of Advanced Inorganic Materials
Journal Volume Year Pages Concerned
MRS Bulletin Special Issue 25[9] 2000 17-25

Author Title of Article
K. OKADA In-situ Zeolite X Coating on Glass Fibers by Soft Solution Process
Journal Volume Year Pages Concerned
Microporous Mesoporous Materials 37 2000 99-105

Author Title of Article
P. SIRIPHANNON Influence of Preparation Conditionson the Microstructure andBioactivity of ƒΏ-CaSiO3 Ceramics
Journal Volume Year Pages Concerned
Journal of Biomedical Materials Research 52 2000 32-39

Author Title of Article
Kiyoshi OKADA Sol-Gel Synthesis of YAG/Alumina Long Fibers from Water Solvent Systems
Journal Volume Year Pages Concerned
J. Europ. Ceram. Soc. 20[2] 2000 561-567

Author Title of Article
Kiyoshi OKADA Concentration Effect of Cs+ Additive on ƒΑ-Al2O3-to-ƒΏ-Al2O3 Phase Transitions
Journal Volume Year Pages Concerned
Mater. Lett. 42[2] 2000 175-178

Author Title of Article
Kiyoshi OKADA Thermal Stability of Coprecipitated Al2O3-SiO2 Xerogels Prepared from Aluminiium Nitrate Nonahydrate and Tetraethylorthosilicate
Journal Volume Year Pages Concerned
J. Ceram. Soc. Jpn. 108[2] 2000 122-127

Author Title of Article
Kiyoshi OKADA Effects of Divalent Cation Additives on the ƒΑ-Al2O3-to-ƒΏ-Al2O3 Phase Transition
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 83[4] 2000 928-932

Author Title of Article
M. ENDO Formation of Formation in the Deep Oxidation of Methanol on Pt(11) under UHV Condition Studied by IRAS
Journal Volume Year Pages Concerned
J. Phys. Chem. B. 104[20] 2000 4916-4922

Author Title of Article
M. HARA Mechano-Catalytic Overall Water Splitting (II) Nafion-Deposited Cu2On
Journal Volume Year Pages Concerned
Appl. Catal. A, General 190 2000 35-42

Author Title of Article
M. HARA A Study of Mechano-Catalysis for Overall Water Splitting
Journal Volume Year Pages Concerned
J. Phys. Chem. B 104[4] 2000 780-785

Author Title of Article
S. ICHIHARA Two Adsorption States of C2H4 at Saturation Coverage on Pd (110)-(2x1)-H
Journal Volume Year Pages Concerned
Chem. Lett. @ 2000 112-113

Author Title of Article
J. N. KONDO IR Characterization of Mesoporous Tantalum Oxide, Ta-TMS-1
Journal Volume Year Pages Concerned
Bull. Chem. Soc. Jpn. 73 2000 1123-1129

Author Title of Article
J. N. KONDO IR Study of Double Bond Migration of 1-Butene on SiO2-Al2O3
Journal Volume Year Pages Concerned
J. Jpn. Petro. Inst. 43[3] 2000 234-240

Author Title of Article
J. N. KONDO (OD) Groups on Ferrierite Zeolite Studied by FT-IR
Journal Volume Year Pages Concerned
Stud. Surf. Sci. Catal. 130 2000 2933-2938

Author Title of Article
J. N. KONDO Acid Property of Silanol ] Groups on Zeolites Assessed by Reaction Probe IR Study
Journal Volume Year Pages Concerned
J. Catal 191 2000 275-281

Author Title of Article
T. MIURA Density Functional Study of Ethylene Hydrogenation on Pt (111) Surface
Journal Volume Year Pages Concerned
J. Phys. Chem. B 104 2000 6809-6814

Author Title of Article
H. TAKAHASHI Synthesis of (H3O) TiNbO5 ₯ 0. 26H2O via Hydroniuim Ion (H3O+) Exchange Reaction and Its Photocatalysic Activity for H2 Evolution from Aqueous Methhanol Solution
Journal Volume Year Pages Concerned
PHys. Chem. Chem. Phys. @ 2000 2

Author Title of Article
T. TAKATA Photocatalytic Water Decomposition by Layered Perovskites
Journal Volume Year Pages Concerned
Stud. Surf. Sci. Catal. 130 2000 2933-2938

Author Title of Article
E. YODA Shape Selective Addsorption of Olefins on Btonsted Acidic OH(OD) Groups on Ferrierite Studied by FT-IR
Journal Volume Year Pages Concerned
Appl. Catal. A: General 194-195 2000 275-283

Author Title of Article
T. SHIMAZAKI Phase Relations in the Pr-Mn-O System at 1000 Ž
Journal Volume Year Pages Concerned
Journal of Materials Science Letters 19 2000 2029-2031

Author Title of Article
Hirotaka FUJIMORI In situ Ultraviolet Raman Study on the phase Transition of Hafnia up to 2085 K
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc 84[3] 2000 663-665

Author Title of Article
S. W. SONG Electrochemically Deposited LiCoO2 Film on Platinum Metal Substrate under Hydrothermal Condition
Journal Volume Year Pages Concerned
Proceeding of PMP-2000 @ 2000 975-978

Author Title of Article
Sergiy KORABLOV Hydrothermal Corrosion of TiN, TiAlN and CrN Films on SUS-304 in 100 MPA Water
Journal Volume Year Pages Concerned
Proceeding of PMP-2000 @ 2000 945-948

Author Title of Article
R. TERANISHI Room-temperature Direct Patterning of Crystalline Inorganic Materials on Organic Substrates by On-site Solution Reaction
Journal Volume Year Pages Concerned
Proceeding of PMP-2000 @ 2000 961-964

Author Title of Article
Y. MORIYOSHI Kinetics of Sintering at a Constant Rate of Heating
Journal Volume Year Pages Concerned
Ceram. Soc. Jpn. 108 2000 S41-48

Author Title of Article
Kiyoshi OKADA Effects of Monovalent Cation Additives ƒΑ-Al2O3-to-ƒΏ-Al2O3 on Phase Transitions
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc. 83[5] 2000 1233-1236

Author Title of Article
Kiyoshi OKADA In-Situ Zeolite X Coating on Glass Fibers by Soft Solution-Process
Journal Volume Year Pages Concerned
Microp. Mesop. Mater. 37[2] 2000 99-105

Author Title of Article
Kiyoshi OKADA Effect of Preparation Conditions on Porous Properties of Coprecipitated Al2O3-SiO2 XerogelsPrepare from Aluminium Nitrate Nonahydrate and Tetracthylorthosilicate
Journal Volume Year Pages Concerned
Microp. Mesop. Mater. 37[4] 2000 355-364

Author Title of Article
Punnama SIRIPHANNON Influence of Preparation Conditions on the Microstructure and Bioactivity of ƒΏ-CaSiO3 Ceramics: Formation of Hydroxy-apatiote in Simulated Body Fluid
Journal Volume Year Pages Concerned
J. Biomed. Mater. Res. 52[1] 2000 32-39

Author Title of Article
Rathindra Nath DAS Influence of Processing Medium on Retention of Specific Surface Area of Gamma-Alumina at Elevated Temperature
Journal Volume Year Pages Concerned
Appl. Catal. B562[1] 2000 1-8

Author Title of Article
Kiyoshi OKADA Uptake of Various Cations by Imperfectly Ordered KAlSiO4 Prepared by Solid-State Reaction of Kaolinite and K2CO3
Journal Volume Year Pages Concerned
J. Ceram. Soc. Jpn. 108[10] 2000 898-903

Author Title of Article
Seung-Wan SONG Effect of 20-200 Ž Fabrication Temperature on Microstructure of Hydrothermally Prepared LiCoO2 Films
Journal Volume Year Pages Concerned
J. Am. Ceram. Soc 83[11] 2000 2839-2844

Author Title of Article
Yury GOGOTSI Hydrothermal Synthesis of Multiwall Carbon Nanotubes
Journal Volume Year Pages Concerned
J. Mater. Res 15[12] 2000 2591-2594

Author Title of Article
Shu-Hong YU Fabrication of Polystyrene/CdS Hybrid Nanocomposites Embedded with CdS Nanowires by a Soft Solution-Processing Route
Journal Volume Year Pages Concerned
Mater. Res. Soc. Symp. Proc 628 2000 @

Author Title of Article
Shu-Hong YU Direct Fabrication of Ferrite MFe2O4(M=Zn, Mg)/Fe Composite Thin Films by Soft Solution Processing
Journal Volume Year Pages Concerned
Chem. of Mater 12[12] 2000 3805-3810

Author Title of Article
Koji-IOKU Observation of OH Ion in Hydroxyapatite by UV Laser Raman Scattering
Journal Volume Year Pages Concerned
Phosphorus Research Bulletin 11 2000 13-18

Author Title of Article
T. FUJIWARA Direct Fabrication of LiCoO2 Films on Papers by Electrodeposition Method with Interfacial Reaction
Journal Volume Year Pages Concerned
The Minerals, Metals & Materials Society @ 2000 935-938

Author Title of Article
V. PETRYKIN Raman Active Modes in Nd2BaCu3Oz Compound
Journal Volume Year Pages Concerned
Physica C 338 2000 151-156

Author Title of Article
M. OSADA Resonant Raman Scattering and Photoinduced Metastability in Oxygen-ficient YBa2CueOx
Journal Volume Year Pages Concerned
Physica C 338 2000 157-160

Author Title of Article
M. OSADA Raman-active Phonons and their Doping Dependence in Spin-ladder Sr14Cu24O41
Journal Volume Year Pages Concerned
Physica C 338 2000 161-165

Author Title of Article
T. ASAI A Novel Aqueous Solution Route to the Low-temperature Synthesis of SrB12Nb2O9 by Use of Water-Soluble Bi and Nb Complex
Journal Volume Year Pages Concerned
J. Alloys and Compounds 309 2000 113-117

Author Title of Article
H. TAKAHASHI Synthesis of (H3O)TiNbO5-0.26H2O via Hydronium Ion (H3O+) Exchange Reaction and its Photocatalytic Activity for H2 Evolution from Aqueous Methanol Solution
Journal Volume Year Pages Concerned
Phys. Chem. Chem. Phys. 2 2000 4461-4464

Author Title of Article
J. FRANTTI Neutron Diffraction Studies of Pb (ZrxTi1-x) O3 Ceramics
Journal Volume Year Pages Concerned
Jpn. J. Appl. Phys. 39 2000 5697-5703

Author Title of Article
Michiko KAMIYA Solid Solution Formation and Crystal Growth of CeO2 Doped with Nd Hydrothermal Condition
Journal Volume Year Pages Concerned
Electrochem. Soc. Proc 99-38 2000 557-567

Author Title of Article
K. Byrappa Hydrothermal Preparation of TiO2 and Photocatalytic Degradation of Hexachlorocyclohexane and Dichlorodiphenyltrichloromethane
Journal Volume Year Pages Concerned
Environmental Technology 21 2000 1085-1090

Author Title of Article
Masahiro YOSHIMURA Soft Processing for Advanced Inorganic Materials
Journal Volume Year Pages Concerned
MRS Bulletin Special Issue 25[9] 2000 12-13

Author Title of Article
Zhibin WU The Formation of Pyrochlore Potassium Tantalate Thin Films by Soft Solution Processing
Journal Volume Year Pages Concerned
Thin Solid Films 375 2000 46-50

Author Title of Article
Yury GOGOTSI Graphite Polyhedral Crystals
Journal Volume Year Pages Concerned
Science 290 2000 317-319

Author Title of Article
Zhibin WU Hydrothermal Formation and Growth of Single- and Double-Layer BaTiO3 and SrTiO33 Films on the Flexible Polymer Film Substrates from Sol-Gel Amorphous Titanium Oxide Films
Journal Volume Year Pages Concerned
Chem. of Mate 12[11] 2000 3356-3361

Author Title of Article
T. KANAZAWA Reaction Chemistry of Hyudrocyapatite: Formation and Decomposition
Journal Volume Year Pages Concerned
Chemistry 49[1] 2000 19-28

Author Title of Article
Y. SHIMIZU The Effect of Temperatures on the Formation of Nanotubes in Nitrogen-Carbon-Nitrogen System
Journal Volume Year Pages Concerned
Trans. Mater. Res. Soc. 25 2000 329-332

Author Title of Article
M. KUKRIHARA Synthesis and Electrochemical Behavior of Porous Carbon Powders Prepared by Thermal Plasma Treatment of Phenolic Resin
Journal Volume Year Pages Concerned
Trans. Mater. Res. Soc. 25 2000 39-42

Author Title of Article
Y. MORIYOSHI The Preparation and characterization of Boron-Carbon- Nitrogen Nanotubes by a cd Arc Plasma
Journal Volume Year Pages Concerned
Processing Materials for Properties, ed. byR. Mishra and C. Yamauchi @ 2000 387-392

Author Title of Article
Y. MORIYOSHI Preparation of Hydroxyapatite in a Reaction between Alite and Phosphoric Acid
Journal Volume Year Pages Concerned
Trans. Mater. Res. Soc. Japan 25 2000 1143-1146

Author Title of Article
Y. MATSUMOTO A New Electrochemical Method to Prepare Meso-Porous Titanium (IV) Oxide Photocatalyst Fixed on Alumite Substrate
Journal Volume Year Pages Concerned
J. Phys. Chem. B 104 2000 4204-4209

Author Title of Article
R. ABE Steady Hydrogen Evolution from Water on Eosin Y Fixed TiO2 Photocatalyst Using Silane-coupling Reagent under Visible Light Irradiation
Journal Volume Year Pages Concerned
J. Mol. Catal. A 137 2000 63-69

Author Title of Article
G. HITOKI Mechano-Catalytic Overall Water Splitting on Some Mixed Oxides
Journal Volume Year Pages Concerned
Catal. Today 63 2000 175-181

Author Title of Article
M. HARA Exfoliation and Photocatalytic Activities of Layered Oxides KSr2Nb3O10
Journal Volume Year Pages Concerned
The Minerals, Metals & Materials Society @ 2000 235-238

Author Title of Article
C. T. K. THAMINIMULLA Effect of Chromium Addition for Photocatalytic OversllWater Splitting onNi-K2La2Ti3O10
Journal Volume Year Pages Concerned
J. Catal 196 2000 362-365

Author Title of Article
J. JIA Selective Hydrogenation of Acetylene Over Au/Al2O3 Catalst
Journal Volume Year Pages Concerned
J. Phys. Chem. B 104[47] 2000 11153-56

Author Title of Article
Y. MATSUMOTO Atomic Force MicroscopyStudy of Layered Titanate HxTi(2-x/4)  x/4 ₯ H2O Films
Journal Volume Year Pages Concerned
Solid-State Lett. 3[10] 2000 481-484

Author Title of Article
S. NISHIO Anomalous Profile of Amplitude Mode in K0.30MoO3 at LowTemperatures Studied by Raman Spectroscopy
Journal Volume Year Pages Concerned
Solid State Communications 116 2000 7-9

Author Title of Article
C. P. UDAWATTE Low-Temperature Synthesis of Pure BaSnO3 and the (Ba1-x) SrxSnO3 Solid-Solutions by the PolymerizedComplex Method
Journal Volume Year Pages Concerned
Solid State Ionics 128 2000 217-226

Author Title of Article
E. A. GOODILIN Filament Crystal Growth in the Systems M-Mn-O (M=Ba, Sr, a) Using Chloride Fluxes
Journal Volume Year Pages Concerned
Dokl. Acad. Nauk. 372 2000 100-104

Author Title of Article
V. V. PETRYKIN Structural Disorder and Superconductivity Suppression in NdBa2Cu3Oz (z-7)
Journal Volume Year Pages Concerned
Physica C 340 2000 16-32

Author Title of Article
H. YASUOKA Hole Concentration of Sintered Bi2-xPbxSr2Ca1-yYyCu2O8+d
Journal Volume Year Pages Concerned
Physica B 284-288 2000 1087-1088

Author Title of Article
M. OSADA Photoinduced Metastability in YBa2Cu3Ox Studied by in-situ Raman Scattering
Journal Volume Year Pages Concerned
Physica B 284-288 2000 681-682

Author Title of Article
K. KAMADA Cation Doping into the Superconducting Bi-Sr-Ca-Cu-O Ceramics Using theSolid Oxide Electrochemical Doping Method
Journal Volume Year Pages Concerned
Electrochemistry 68[6] 2000 540-542

Author Title of Article
Y. MATSUMOTO Electrochemical and Photoelectrochemical Processing for Oxide Films
Journal Volume Year Pages Concerned
MRS Bulliten 25[9] 2000 47-50

Author Title of Article
M. KOINUMA Atomic Force Microscopy Study of Layered Titanate HxTi(2-x/4) nH2O Films
Journal Volume Year Pages Concerned
Electrochem. Solid-State Lett. 3[10] 2000 481-484

Author Title of Article
Takashi ISHIHARA Room Temperature Growth of Magnetite Films on Arachic Acid Monomolecular Layered
Journal Volume Year Pages Concerned
The Korean Journal of Ceramics 6[4] 2000 401-404

Author Title of Article
Fumio SHIRASAKI Evaluation of Spin Directionin Ferrite-Plated Films by Fe57 Conversion Eelctron Mossbauer Spectroscopy
Journal Volume Year Pages Concerned
The Korean Journal of Ceramics 6[4] 2000 405-407

Author Title of Article
K. KOMEN Observation of Unstable Reaction Intermediate byPicosecond Tunable Infrared Laser Pulses
Journal Volume Year Pages Concerned
Stud. Surf. Sci. Catal. 130 2000 365-370

Author Title of Article
Kyoshi OKADA Characterization of the State of Ni2+ in Ni-exchanged KAlSiO4 by XPS, XRF, XRD, EXAFS, and NMR
Journal Volume Year Pages Concerned
J. Ceram. Soc. Jpn. 108[11] 2000 989-992

Author Title of Article
M. KAKIHANA The Synthesis of Photocatalysts Using the Polymerizable- Complex Method
Journal Volume Year Pages Concerned
MRS Bulletin 25 2000 27-32

Author Title of Article
S. YAMAMOTO A Polymer Complex Solution Route to the Low-Temoperature Synthesis of Tetragonal Zr0.88Ce0.12O2 with a Reduced Ammount of Organic Subtance
Journal Volume Year Pages Concerned
J. Alloysand Compounds 297 2000 81-86

Author Title of Article
H. FUJIMORI Phase Transition and Soft Phonon Modes in SrZrO3 Around 1200Ž by Ultraviolot Laser Raman Spectroscopy
Journal Volume Year Pages Concerned
Physical Review B 61 2000 3971-3974

Author Title of Article
J. BACKSTROM Raman Scattering in YBa2Cu4O8 and PrBa2Cu4O8: Indications of Pseudogap Effects in Nonsuperconducting PrBa2Cu4O8
Journal Volume Year Pages Concerned
Physical Review B 61 2000 7049-7054

Author Title of Article
M. KAKIHANA Raman Slpectroscopy as a Unique Tool for Characterizing High-Tc Superconducting zoxides
Journal Volume Year Pages Concerned
Physical C 338 2000 144-150

Author Title of Article
S. TOCHIHARA Magnetic Response of Y/Pb Doped Single-Crystal Bi2Sr2CaCu2O8+d Superconductors
Journal Volume Year Pages Concerned
IEEE Trans. Appl. Superconductivity 14A 2000 19-24

Author Title of Article
S. WADA Charge of Macroscopic and Microscopic Symmetries in Relaxor PZN SingleCrystal under DC-bias Field
Journal Volume Year Pages Concerned
Trans. Mat. Res. Soc. Jpn. 14A 2000 19-24

[Reference Books]
Author Title of Book
K. BYRAPPA Handbook of Hydrothermal Technology
Publisher Year Pages
William Andrew Publishing 2000 870


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